Non-ideal effects in organic-inorganic materials for gas separation membranes

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Maximizing the right stuff: The trade-off between membrane permeability and selectivity (2017, background): “However, most experimental results fall below the theoretical maximum because of unfavorably large interfacial gaps between the dispersed nanomaterials and polymermatrix and relatively limited dispersed phase loading due to particle agglomeration (79).”
High pressure gas separation performance of mixed-matrix polymer membranes containing mesoporous Fe(BTC) (2014, background): “Knowledge of the thermal stability of the MOF and MMMs is of importance for both high temperature gas separation applications and because heating of the polymer above its Tg or thermal annealing is often applied to improve the properties of the membranes [60,61].”