Correlating Li+ Solvation Sheath Structure with Interphasial Chemistry on Graphite

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The influence of FEC on the solvation structure and reduction reaction of LiPF6/EC electrolytes and its implication for solid electrolyte interphase formation (2019, background): “We find weak to little dependence of the reduction potential on the number of explicitly coordinating solvents [59,109], e.”
Uncharted Waters: Super-Concentrated Electrolytes (2020, background): “It was this new chemical reliance of interphase on anion instead of solvent molecules that lifts the many traditional confinements imposed on electrolyte design, the most conspicuous of which is ethylene carbonate (EC), the indispensable solvent in electrolytes for any LIBs manufactured nowadays, pr”
Review on modeling of the anode solid electrolyte interphase (SEI) for lithium-ion batteries (2018, methodology): “Combined with this chemical information, e Peled6 pictured SEI as a mosaic structure and translated it into an equivalent circuit model in 1997 (Copyright: The Electrochemical Society). f Aurbach et al.7 illustrated the formation process of SEI starting from electrolyte reduction on electrode surfac”