Landau damping of quantum plasmons in metal nanostructures

By Xiaoguang Li, Di Xiao, Zhenyu Zhang. 2013

158 citations recorded by the source corpus.

Using the random phase approximation with both real space and discrete electron–hole (e–h) pair basis sets, we study the broadening of surface plasmons in metal structures of reduced dimensionality, where Landau damping is the dominant dissipation channel and presents an intrinsic limitation to plasmonics technology. We show that for every prototypical class of systems considered, including zero-dimensional nanoshells, one-dimensional coaxial nanotubes and two-dimensional ultrathin films, Landau damping can be drastically tuned due to energy quantization of the individual electron levels and e–h pairs. Both the generic trend and oscillatory nature of the tunability are in stark contrast with the expectations of the semiclassical surface scattering picture. Our approach also allows to vividly depict the evolution of the plasmons from the quantum to the classical regime, and to elucidate the underlying physical origin of hybridization broadening of nearly degenerate plasmon modes. These findings may serve as a guide in the future design of plasmonic nanostructures of desirable functionalities.

Subfields: Atomic and Molecular Physics, and Optics, Biomedical Engineering, Electronic, Optical and Magnetic Materials

View Paper: https://www.semanticscholar.org/paper/c1d51d2cb9c86141e0f781e242866be3dc2e1f37

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In Atomic and Molecular Physics, and Optics

  1. A. Govorov
  2. Richard V. Craster
  3. S. A. Maier
  4. Prineha Narang
  5. Gregory Hartland

In Biomedical Engineering

  1. Vincenzo Giannini
  2. Prineha Narang
  3. Richard V. Craster
  4. Jamie M. Fitzgerald
  5. A. Govorov
  6. Gregory Hartland
  7. S. A. Maier
  8. Pierre Berini

In Electronic, Optical and Magnetic Materials

  1. Prineha Narang
  2. A. Govorov
  3. Vincenzo Giannini
  4. L. Besteiro
  5. Richard V. Craster
  6. Jamie M. Fitzgerald
  7. Gregory Hartland
  8. S. A. Maier

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