First-principles analysis of electron-phonon interactions in graphene

By K. M. Borysenko, J. Mullen, E. A. Barry, S. Paul, Y. Semenov, J. Zavada, Marco Buongiorno Nardelli, Ki Wook Kim. 2009

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The electron-phonon interaction in monolayer graphene is investigated using density-functional perturbation theory. The results indicate that the electron-phonon interaction strength is of comparable magnitude for all four in-plane phonon branches and must be considered simultaneously. Moreover, the calculated scattering rates suggest an acoustic-phonon contribution that is much weaker than previously thought, revealing an important role of optical phonons even at low energies. Accordingly it is predicted, in good agreement with a recent measurement, that the intrinsic mobility of graphene may be more than an order of magnitude larger than the already high values reported in suspended samples.

Subfields: Materials Chemistry

View Paper: https://www.semanticscholar.org/paper/af19675bf462c26f02eaf6297d7520956fee85ef

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