Wearable energy-dense and power-dense supercapacitor yarns enabled by scalable graphene–metallic textile composite electrodes

By Libin Liu, You Yu, Casey Yan, Kan Li, Zijian Zheng. Nature Communications, 2015

614 citations recorded by the source corpus.

One-dimensional flexible supercapacitor yarns are of considerable interest for future wearable electronics. The bottleneck in this field is how to develop devices of high energy and power density, by using economically viable materials and scalable fabrication technologies. Here we report a hierarchical graphene–metallic textile composite electrode concept to address this challenge. The hierarchical composite electrodes consist of low-cost graphene sheets immobilized on the surface of Ni-coated cotton yarns, which are fabricated by highly scalable electroless deposition of Ni and electrochemical deposition of graphene on commercial cotton yarns. Remarkably, the volumetric energy density and power density of the all solid-state supercapacitor yarn made of one pair of these composite electrodes are 6.1 mWh cm−3 and 1,400 mW cm−3, respectively. In addition, this SC yarn is lightweight, highly flexible, strong, durable in life cycle and bending fatigue tests, and integratable into various wearable electronic devices. It is challenging to fabricate flexible and wearable supercapacitors with high energy and power densities using cost-effective materials and scalable processes. Here, the authors present a supercapacitor yarn based on graphene and metallic textile composites, which shows potential to fulfil those requirements.

Subfields: Biomedical Engineering, Electronic, Optical and Magnetic Materials, Polymers and Plastics

View Paper: https://www.semanticscholar.org/paper/ab07570b4c9a0ac955c157ac6c565bc241586063

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In Biomedical Engineering

  1. K. Novoselov
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In Electronic, Optical and Magnetic Materials

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