Distorted perovskite witheg1configuration as a frustrated spin system

By Tatsumi Kimura, Sumio Ishihara, H. Shintani, Taka-hisa Arima, Kei Takahashi, K. Ishizaka, Y. Tokura. 2002

410 citations recorded by the source corpus.

The evolution of spin- and orbital-ordered states has been investigated for a series of insulating perovskites $R{\mathrm{MnO}}_{3}$ $(R=\mathrm{L}\mathrm{a},\mathrm{P}\mathrm{r},\mathrm{N}\mathrm{d},\dots{}).$ $R{\mathrm{MnO}}_{3}$ with a large ${\mathrm{GdFeO}}_{3}$-type distortion is regarded as a frustrated spin system having ferromagnetic nearest-neighbor and antiferromagnetic (AF) next-nearest-neighbor (NNN) interactions within a ${\mathrm{MnO}}_{2}$ plane. The staggered orbital order associated with the ${\mathrm{GdFeO}}_{3}$-type distortion induces the anisotropic NNN interaction, and yields unique sinusoidal and up-up-down-down AF ordered states in the distorted perovskites with ${e}_{g}^{1}$ configuration.

Subfields: Condensed Matter Physics, Electronic, Optical and Magnetic Materials

View Paper: https://www.semanticscholar.org/paper/932108a8948948fd8161a51d3cfd72e55e5db168

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In Condensed Matter Physics

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