Al environment in tectosilicate and peraluminous glasses: A 27Al MQ-MAS NMR, Raman, and XANES investigation

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Amorphous materials: Properties, structure, and durability: Structure of Mg- and Mg/Ca aluminosilicate glasses: 27Al NMR and Raman spectroscopy investigations (2008, background): “Quantification of the abundance of these species in peraluminous CaO-Al2O3-SiO2 (CAS) glasses shows a strong preference for the formation of VAl (Sen and Youngman 2004; Neuville et al. 2004a, 2006).”
A computer simulation study of natural silicate melts. Part I: Low pressure properties (2007, result): “These results are in agreement with spectroscopic data on alkaline-earth aluminosil-icate glasses of related compositions (Wu et al., 1999; Neuville et al., 2004) which show a signiﬁcant contribution of [5] Al.”
Letter. Aluminum coordination and the densification of high-pressure aluminosilicate glasses (2005, background): “This has also been observed in an ambi- ent pressure Na3AlSi7O17 glass (Allwardt et al. 2005a) as well as for several aluminosilicates with much lower NBO contents (Toplis et al. 2000; Stebbins et al. 2000; Neuville et al. 2004).”