Strained Bubbles in van der Waals Heterostructures as Local Emitters of Photoluminescence with Adjustable Wavelength
By A. Tyurnina, D. Bandurin, E. Khestanova, V. Kravets, M. Koperski, Francisco Guinea, A. Grigorenko, A.K. Geim, I. Grigorieva. ACS Photonics, 2019
146 citations recorded by the source corpus.
The possibility to tailor photoluminescence (PL) of monolayer transition metal dichalcogenides (TMDCs) using external factors such as strain, doping, and external environment is of significant interest for optoelectronic applications. Strain in particular can be exploited as a means to continuously vary the band gap. Micrometer-scale strain gradients were proposed for creating “artificial atoms” that can utilize the so-called exciton funneling effect and work, for example, as exciton condensers. Here we describe room-temperature PL emitters that naturally occur whenever monolayer TMDC is deposited on an atomically flat substrate. These are hydrocarbon-filled bubbles, which provide predictable, localized PL from well-separated sub-micrometer areas. Their emission energy is determined by the built-in strain controlled only by the substrate material, such that both the maximum strain and the strain profile are universal for all bubbles on a given substrate, i.e., independent of the bubble size. We show that ...
Subfields: Materials Chemistry
View Paper: https://www.semanticscholar.org/paper/612729b7b813a9ba41decb9ea16a76887713478d
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In Materials Chemistry
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- Strain engineering of two‐dimensional materials: Methods, properties, and applications (2021, background): “(E) AFM image (The scale bar was 2 μm) and (F) cross-sectional height profile of a typical bubble formed at the interface.(77) Reproduced with permission: Copyright 2019, American Chemical Society.”