Effects of Inhomogeneities—Nanoscale to Mesoscale—on the Durability of Li-Ion Batteries

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Tortuosity in electrochemical devices: a review of calculation approaches (2018, background): “microstructures in this field to prevent spatial distribution of performance and degradation [155].”
Rethinking How External Pressure Can Suppress Dendrites in Lithium Metal Batteries (2019, background): “Li protrusions can also penetrate through the separator and cause a short circuit [3, 7-11], potentially resulting in a fire [12].”
Modeling of internal mechanical failure of all-solid-state batteries during electrochemical cycling, and implications for battery design (2017, background): “[59] observed (by digital image correlation techniques) in graphite electrodes, where most of graphite’s swelling was compensated by reducing the electrode porosity.”
Microstructural Evolution of Battery Electrodes During Calendering (2020, background): “5% calendered AM_L with three distinct properties (1) as-prepared electrode; (2) faster solid-state diffusion Ds_f; (3) faster reaction kinetics Rk_f (i.”
The state of understanding of the lithium-ion-battery graphite solid electrolyte interphase (SEI) and its relationship to formation cycling (2016, background): “The right column images are higher magnification (100,000×) of the images in left column (30,000×).[56] “Reprinted (adapted) with permission from (Harris, S.”