Gas uptake and chemical aging of semisolid organic aerosol particles

By M. Shiraiwa, M. Ammann, Thomas Koop, Ulrich Pöschl. Proceedings of the National Academy of Sciences of the United States of America, 2011

648 citations recorded by the source corpus.

Subfields: Atmospheric Science, Health, Toxicology and Mutagenesis

View Paper: https://www.semanticscholar.org/paper/14f5f3a2a03ea060e19c2ea5a6497d1d93671d16

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Citations in the corpus

The deposition ice nucleation and immersion freezing potential of amorphous secondary organic aerosol: Pathways for ice and mixed‐phase cloud formation (2012, methodology): “…explanation for this behavior is that water uptake is more affected by the lower DH2O at lower temperatures which results in slower diffusion of water molecules into the first particle layers [Koop et al., 2011; Shiraiwa et al., 2011; Zobrist et al., 2011] irrespective of particle bulk O/C ratio.”
Modeling the formation and growth of atmospheric molecular clusters: A review (2020, background): “Phase state, e.g. solid/liquid: The phase state of larger particles is an area of intense research, see (Pöschl & Shiraiwa, 2015; Reid et al., 2018; Shiraiwa et al., 2011, 2017; Virtanen et al., 2010) and will not be discussed here.”
Competition between water uptake and ice nucleation by glassy organic aerosol particles (2014, neutral): “Also, in the glassy state, the organic molecules diffuse on a much longer timescale compared to the experimental timescale of minutes to hours (cf. Shiraiwa et al., 2011; Koop et al., 2011).”
Predicting the glass transition temperature and viscosity of secondary organic material using molecular composition (2017, background): “The particle phase state, viscosity, and bulk diffusivity have been shown to affect the gas uptake and chemical transformation of organic compounds due to the kinetic limitations of bulk diffusion (Shiraiwa et al., 2011; Abbatt et al., 2012; Kuwata and Martin, 2012; Zhou et al., 2013; Slade and Knop”